The 30-year-old, who still has a year to run on his Ulster contract, will join the Exiles this summer.
Humphreys has been inconsistent this season and failed to make the Ulster line-up for the Heineken Cup semi-final win over Edinburgh last weekend.
Shane Geraghty's return to London Irish provides stiff competition for Humphreys to secure a starting spot.
Geraghty, a product of the Exiles' academy, left the club for Northampton in 2009.
The 27-year-old spent two seasons at Franklin's Gardens before moving to France to play for Brive.
Humphreys returned to Ulster from the Tigers in 2008 and has scored 617 points in 81 games for the province.
OSM news service
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